there is a user settings tool in codeplex to manage some of the settings.
https://crm2011usersettings.codeplex.com/
the xrmtoolbox has a feature to change outlook filters for each user in bulk.
https://xrmtoolbox.codeplex.com/
regards
Jithesh
Take a look at this.
http://msdn.microsoft.com/en-us/library/gg328205.aspx
Jason Peterson
I have the xrmtoolbox, however I dont see the option to change the contact sync options (see photo)